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This paper reports results from an experiment designed to measure the nascent rovibrational population of H2 molecules that have formed through the heterogeneous recombination of H atoms on the surface of cosmic dust analogues under
conditions approaching those of the interstellar medium (ISM). H2 that has formed on a highly oriented pyrolytic graphite (HOPG) surface has been detected, using laser induced resonance-enhanced
multi-photon ionization (REMPI), in the v = 1 (J= 0–3) rovibrational states at surface temperatures of 30 K and 50 K. These excited product molecules display rotational temperatures
significantly higher than the target surface temperature. These first results suggest that a considerable proportion of the
binding energy released on formation of the H2 is deposited in the surface, in addition to internal excitation of the product molecules.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
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O. J. Bennett A. S. Dickinson T. Leininger F. X. Gadéa 《Monthly notices of the Royal Astronomical Society》2003,341(1):361-368
The role in radiative association of narrow resonances arising from quasi-bound levels is examined. For the rate coefficient the contribution from such levels is readily calculated in terms of the Einstein A -coefficient from bound rovibrational levels generated using a suitable alternative boundary condition. By locating systematically all the quasi-bound levels, an enhancement by more than an order of magnitude of the rate coefficient for Li(2s) + H(1s) association above about 600 K is obtained. The effect on the LiH abundance in the early Universe is no more than an increase of a factor of 3 for limited ranges of values of the redshift. For the Li(2p) state the effect of narrow resonances appears to have been taken into account in previous calculations. 相似文献
15.
Ramona Núñez-López Anton Lipovka Vladimir Avila-Reese 《Monthly notices of the Royal Astronomical Society》2006,369(4):2005-2012
Possible detection of signatures of structure formation at the end of the 'dark age' epoch ( z ∼ 40–20) is examined. We discuss the spectral–spatial fluctuations in the cosmic microwave background radiation (CMBR) temperature produced by elastic resonant scattering of CMBR photons on deuterated hydrogen (HD) molecules located in protostructures moving with peculiar velocity. Detailed chemical kinematic evolution of HD molecules in the expanding homogeneous medium is calculated. Then, the HD abundances are linked to protostructures at their maximum expansion, whose properties are estimated by using the top-hat spherical approach and the Λ cold dark matter (ΛCDM) cosmology. We find that the optical depths in the HD three lowest pure rotational lines for high-peak protohaloes at their maximum expansion are much higher than those in LiH molecule. The corresponding spectral–spatial fluctuation amplitudes, however, are probably too weak to be detected by current and forthcoming millimetre telescope facilities. We extend our estimates of spectral–spatial fluctuations to gas clouds inside collapsed CDM haloes by using results from a crude model of HD production in these clouds. The fluctuations for the highest peak CDM haloes at redshifts ∼20–30 could be detected in the future. Observations will be important to test model predictions of early structure formation in the Universe. 相似文献
16.
Z. Q. Qu C. L. Xu X. Y. Zhang X. L. Yan C. L. Jin 《Monthly notices of the Royal Astronomical Society》2006,370(4):1790-1796
The influence of magnetic fields on the energy level populations of atoms is firstly studied by analysing the Stokes profiles of Fe i 6302.5 forming in the solar magnetized atmosphere, with the aid of a departure factor defined to evaluate the deviation from the normal Boltzmann distribution without a magnetic field. This factor is directly related to the ratio of line-source function to the continuum one. The relationship between the departure and the magnetic field reveals an effect that the magnetic field induces an exponential increase in the level population of the lower level of Fe i 6302.5 (Landé factor g = 2.5 ) with the field strength. This indicates that the magnetic field can cause the redistribution of populations of those levels whose Landé factors are non-zero. Therefore, this effect should be included in the calculation of the statistical equilibrium. Secondly, an experiment utilizing the Hg5461 line in the laboratory on the Earth is carried out to reveal that the exponential relation is independent of variations in temperature, and the excitation is completely magneto-induced. Finally, the exponential relation is explained by taking account of the magnetic energy in the Boltzmann distribution. 相似文献
17.
E. Biémont P. Palmeri P. Quinet G. Paquin Z. G. Zhang G. Somesfalean S. Svanberg 《Monthly notices of the Royal Astronomical Society》2001,328(4):1085-1090
Lifetimes of six levels belonging to the 4f10 6p configuration of Ho iii have been measured for the first time using the time-resolved laser-induced fluorescence method. They are compared with multiconfigurational pseudo-relativistic Hartree–Fock calculations. A very good agreement is found. Using the experimental lifetimes and theoretical branching fractions, a first set of transition probabilities of astrophysical interest has been obtained for this ion. 相似文献
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Univariate and multivariate stress release models are fitted to historical earthquake data from North China. It is shown that a better fit is obtained by treating separately the Eastern part of the region, including the North China Plain and Bohai Sea, and the Western part of the region, including the Ordos Plateau and its Eastern boundary. Further improvement is obtained by fitting the large events (M7.6) and smaller events in the Western region by different stress release models. The comparisons are made by computing the likelihoods of the fitted models and discounting the number of parameters used by Akaike's AIC criterion. The models are used to develop long-term risk scenarios for the East and West regions. 相似文献
20.
海相碳酸盐岩层系不整合量化研究及其意义——以四川盆地北部二叠系为例 总被引:2,自引:1,他引:1
本文以四川盆地北部二叠系为例,将层序地层分析和沉积盆地波动过程分析相结合,提出了运用沉积波动过程分析研究沉积记录不完整性的量化方法,该方法可以相对准确地定量描述盆地形成演化过程中的升降运动,恢复无地层"记录"中的沉积-剥蚀过程,进而定量分析盆地的沉积-剥蚀过程、计算沉积间断(不整合)内的地层剥蚀量、认识其时空分布规律.同时,通过实际钻井及"人工井"的波动过程分析,结合地震剖面解释成果,可以作出主要不整合的空间分布图、各层位的剥蚀厚度图和原始厚度图、各期构造的剥蚀量分布图等重要基础图件,为盆地进一步系统分析及盆地模拟打好基础,结合沉积相研究及构造样式分析还可分析盆地沉积中心、生油层、盖层、储层等在时空中的变化规律.由于沉积盆地的升降波动过程直接影响着盆地的埋藏史、热史和生、排烃史,因此通过沉积波动过程的系统分析不仅能正确建立盆地演化的地质模型,还可以正确认识油气形成与分布规律,有效指导油气勘探. 相似文献